Influence of solar activity on ambient dose equivalent H*(10) measured with thermoluminescent dosimeters in Slovenia.

Ambient dose equivalent H*(10) is measured to assess general population exposure to ionising radiation. From its spatial and time variations it is possible to identify sources of exposure. In Slovenia, semi-annual H*(10) is measured routinely with thermoluminescence dosimeters at 66 locations around the Nuclear Power Plant (NPP) Krsko and at 50 other locations covering the rest of Slovenian territory. Since the Chernobyl accident contamination had ceased to contribute to ambient dose equivalents, we have been calculating correlation coefficients between annual mean number of sunspots and annual H*(10). These correlation coefficients were calculated for five locations in western Slovenia and for five annual H*(10) extracted from measurements around NPP Krsko. Their ranges between -0.64 and -0.38 suggest a clear negative correlation between solar activity and H*(10). Mean annual H*(10) averted by solar activity in the past two solar maxima reached 0.070 mSv around NPP Krsko (155 m.a.s.l.) and 0.132 mSv and 0.180 mSv at Kredarica (2515 m.a.s.l.). Quantifying the influence of the solar activity on the ambient dose equivalent helps us to better understand exposure of the general population to ionising radiation.

Measurement uncertainty arising from sampling of environmental samples.

In 2017, a new revision of the ISO/IEC 17025 standard was issued. One of the important changes is that the uncertainty arising from sampling has to be evaluated. Based on this new requirement, we evaluated the contribution of the sampling procedure to the total uncertainty budget of the high-resolution gamma-ray spectrometry of environmental soil, tap water and aerosol filter samples. We performed statistical analyses of measurements of sets of samples taken from the same target in the same general time period. The determination of sampling uncertainty was based on the evaluation of the standard deviation of the set of measurement results and the combined uncertainty budget of sample preparation and analysis. When the spatial and temporal heterogeneities are low, the sampling uncertainty is estimated to be around 5% (k = 1) for soil samples and 30-40% (k = 1) for air samples. For single tap water samples collected consecutively, sampling uncertainty does not have a significant contribution to the complete uncertainty budget.

Negative correlation between the number of sunspots and the occurrence of 7Be and 22Na in the surface air and their contribution to radiation doses.

This article presents yearly mean concentrations of cosmogenic radionuclides 7Be and 22Na occurring in dry and wet depositions (fallout) and aerosols. Time dependencies negatively correlated with the yearly mean number of sunspots. Activity concentrations of 7Be and 22Na in aerosols in the surface air had a correlation of near-unity. 7Be in aerosols exhibited a smoother time dependence than 22Na, implying that the production of 22Na is more sensitive to the solar activity than the production of 7Be. The effect of the measured doses on the general population through internal and external exposure to radiation from cosmogenic radionuclides was small.

Systematic influences of gamma-ray spectrometry data near the decision threshold for radioactivity measurements in the environment.

Several methods for reporting outcomes of gamma-ray spectrometric measurements of environmental samples for dose calculations are presented and discussed. The measurement outcomes can be reported as primary measurement results, primary measurement results modified according to the quantification limit, best estimates obtained by the Bayesian posterior (ISO 11929), best estimates obtained by the probability density distribution resembling shifting, and the procedure recommended by the European Commission (EC). The annual dose is calculated from the arithmetic average using any of these five procedures. It was shown that the primary measurement results modified according to the quantification limit could lead to an underestimation of the annual dose. On the other hand the best estimates lead to an overestimation of the annual dose. The annual doses calculated from the measurement outcomes obtained according to the EC's recommended procedure, which does not cope with the uncertainties, fluctuate between an under- and overestimation, depending on the frequency of the measurement results that are larger than the limit of detection. In the extreme case, when no measurement results above the detection limit occur, the average over primary measurement results modified according to the quantification limit underestimates the average over primary measurement results for about 80%. The average over best estimates calculated according the procedure resembling shifting overestimates the average over primary measurement results for 35%, the average obtained by the Bayesian posterior for 85% and the treatment according to the EC recommendation for 89%.

Evaluation of comparison and proficiency test results of gamma ray spectrometry at Jozef Stefan Institute from 1986 to 2014.

One of the best ways to demonstrate the performance and capabilities of testing laboratories is to participate successfully in different international comparison schemes and proficiency tests. The overview of all results of such schemes in the field of high resolution gamma-ray spectrometry where the Laboratory for Radioactivity Measurements (LMR) of the Jozef Stefan Institute (JSI), Slovenia, participated in years 1986-2014 is presented. Different schemes are compared, strong points and drawbacks of different providers and schemes regarding evaluation procedures, determination of reference values, reporting time, sets of radionuclides included in the samples and range of activities of different radionuclides are discussed. One of the main conclusions is that the comparison and proficiency test samples normally contain substantially larger activities than are usually detected in environmental samples. Therefore the capability of determination of activities close to detection limits is usually covered only by few schemes.

An analysis of the causes of discrepant results in proficiency tests in a testing laboratory.

We present an analysis of the results reported in the framework of proficiency tests performed in the years 2003-2007 in a gamma-ray spectrometry laboratory. Measurements of 102 samples and 622 results reporting the activities or activity concentrations of 39 gamma- or X-ray emitters are included in the study. A total of 61 results were found to be in disagreement with their target values. The cause of the disagreement was not found for only 21 discrepant results.

A method for calculation of true coincidence summing correction factors for extended sources.

In gamma-ray spectrometry, true coincidence summing correction factors for an extended sample can be calculated from full-energy-peak and total efficiencies as if the sample were a point source, if the so-called linear-to-square- (LS) curve, introduced by Blaauw and Gelsema, is known and properly applied. A method is described for obtaining the efficiencies and the corresponding LS-curve for an arbitrary cylindrical sample from calibration measurements in a reference geometry. The approach is aimed at the analysis of samples measured on p-type HPGe detectors in environmental gamma-ray spectrometry and was successfully verified against experimental data.